Aerosols
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The ACES (Aerosol Coupling in the Earth System) project was an integrated research programme that aims to reduce uncertainties in our fundamental understanding of the formation of BSOA (Biogenic Secondary Organic Aerosol) and the subsequent impact on atmospheric composition, through coordinated chamber studies, field studies, process model development, and application of atmospheric models of chemistry and transport to assess coupling and feedbacks in the Earth system. As part of the APPRAISE-ACES project, the University of Manchester carried out several field measurements studies in the rainforest in Borneo (based at the forest in-canopy site located at the FACE (Forests Absorbing CO2 Emissions) nursery at the Sabahmas Estate oil plantation in Malaysia) and also aerosol chamber studies which followed in Manchester. This dataset collection contains measurements from aerosol instruments used in Borneo including Condensation Particle Counter (CPC), Grimm Optical Particle Counter (Grimm), Scanning Mobility Particle Sizer (SMPS) and a Sonic Anemometer 1. The ACES field measurement programme was designed to develop the objectives of the Oxidant and Particle Photochemical Processes above a South-East Asian Tropical Rain Forest (OP3-Danum-08) project.
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This data was collected as a result of the FIRETRACC/100 (Firn Record of Trace Gases Relevant to Atmospheric Chemical Change over 100 yrs) project conducted in 1998 and 1999. The FIRETRACC project aimed to determine the history of numerous trace gases of both human (pollution) and natural origin over the 20th century in the global atmosphere. This was achieved by pumping old air out of deep unconsolidated snow (known as firn) that accumulates to depths of around 50 to 100 m on the polar ice caps of both hemispheres. The resulting firn air samples from the Arctic and Antarctic were returned to Europe and the US for multiple gas and isotope analysis in a number of research laboratories. The firn air samples were analysed for well over eighty separate trace gases (halocarbons, non-methane hydrocarbons, alkyl nitrates, sulphur species, etc.), and thirteen different isotopic measurements of CO2, CH4, CO and permanent gases (O2, N2, Ar, Kr). In summary, the objectives of FIRETRACC/100 are as follows: * To determine the global trends of trace gases relevant to troposphericchemistry over the 20th century. These will include CO, the isotopiccomposition of CO, hydrocarbons, alkyl nitrates, numerous OH-reactivehalocarbons (such as methyl chloride, methyl chloroform, methyl bromide,hydrochlofluorocarbons, etc.), and sulphur gases (COS, CS2, etc.). Trends of longer lived gases will also be determined for dating purposes (CO2, CFCs,SF6, perfluorocarbons, etc.) * Determine the evolution of inter-hemispheric ratios of OH-sensitive species to constrain modelled global OH fields * Examine ratios of parent hydrocarbons to alkyl nitrates to place constraints on NOX fields in models * Elucidate the sources of CO from isotopic studies and use to deconvolute CO/methane coupling in models * Reconstruct the history of ozone, OH and tropospheric oxidising capacity over the past 100 years using full chemistry 2-D models * Determine the influence of 20th century industrialisation on the gas phase composition and chemistry of the lower atmosphere The data consists of ‘primary’ data comprising simple concentration versus depth profiles, and for selected gases also ‘secondary’ data comprising reconstructed historical trends. The firn diffusion model, used in the model reconstruction, is also available through this site.
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This data was collected from the Stratosphere-Troposphere Exchange Project (STEP) conducted onboard the NASA ER-2 aircraft in January and February, 1987 based in Darwin, Australia. This mission was the last of 6 STEP missions which began with the Global Tropospheric Experiment (GTE) in April 1984. The Darwin, Australia phase of STEP utilized 15 instruments and accessed the world's highest, coldest tropopause as well as the largest penetrating cumulonimbus anvils. The flights were designed to test a dehydration mechanism proposed by Danielsen (1982), as well as to acquire sufficient data to test and develop other hypotheses. The STEP missions were designed to investigate different aspects of stratosphere-troposphere exchange (in mass, trace gases, and aerosols), including cloud-free and cloud-dominated mechanisms in both the mid-latitudes and the tropics. STEP was carried out under NASA and the National Oceanic Atmospheric Administration (NOAA). Data from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.
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Data from the flight 7 of 17 from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.
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Data from the flight 3 of 17 from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.
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The European Arctic Stratospheric Ozone Experiment is a European Commission (EC) measurement campaign undertaken in the Northern Hemisphere winter of 1991-92 to study ozone chemistry and dynamics. This dataset contains vertical column measurements of NO, NO2, CH4, O3, HF, HCl, ClONO2, HNO3, CFC-11 and CFC-12 from the BRUKER IFS 120M FTIR spectrometer.
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The European Arctic Stratospheric Ozone Experiment is a European Commission (EC) measurement campaign undertaken in the Northern Hemisphere winter of 1991-92 to study ozone chemistry and dynamics. This dataset contains vertical column measurements of NO2, O3 and OClO.
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Data from the flight 8 of 17 from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.
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Data from the flight 2 of 17 from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.
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Data from the flight 11 of 17 from the NASA/NOAA aircraft campaign based in Darwin, Australia in January and February 1987. Designed to investigate mechanisms of equatorial stratosphere-troposphere exchange. Measurements include trace gases and aerosol in cloud free and cloud dominated conditions. This dataset is public.