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This dataset contains measurements of dispersed Nitric Oxide (NO) made at a relatively low traffic area, Mansfield Road, in the city of Oxford, U.K. as part of project funded through the TRANSITION AIR QUALITY Network. NO was released from a bottle with a known concentration of 10,000ppm NO in nitrogen mounted at the back of an electric van and the dispersed NO measured at the roadside using fast response sensors provided by Cambustion Ltd. These measurements were then used to validate Computational Fluid Dynamics Models. The tests were carried out during a single day at different locations on the road. Wind direction, wind speed and the concentration of sensed NO are recorded and presented in the archived dataset.